Carrie Yang   Associate professor

杨晓红,东北大学冶金学院副教授,博士生导师。2014年毕业于澳大利亚新南威尔士大学材料科学与工程学院获工学博士学位,2015年5月回国任职于东北大学冶金学院,在冶金工程博士后流动站从事博士后研究工作,2017年起任东北大学冶金学院讲师、副教授。主要研究方向为光电催化能量转换技术,高级氧化技术与工艺,固废资源的提纯与回收等。作为项目负责人先后主持中国博士后基金,东北大学博士后基金,青年教师科研创新基金,中国自...Detials

Carbon Nanodots Doped Graphite Carbon Nitride Towards Highly Efficient Visible Light Driven-Photocatalytic Hydrogen Evolution

Release time:2024-03-18  Hits:

  • Journal:International Conference on Development and Application of Carbon Nanomaterials in Energetic Materials
  • Abstract:Graphite carbon nitride (g-C3N4), as one of the promising candidates for photocatalytic hydrogen evolution, owns the advantages of visible light response, good stability, and no harm to the environment. However, the photocatalytic water splitting of g-C3N4 has been limited due to its slow photocarrier transfer rate and insufficient light absorption. Herein, carbon dots (CDs) were prepared by a hydrothermal method using ginkgo biloba leaves as the raw material. Afterwards, the g-C3N4 nanosheets decorated with CDs were obtained by a thermal polymerization method. CDs have unique way of light-induced charge transfer and special heterogeneous interface. The reservoir characteristics of the composite enable to greatly reduce the recombination of photo-generated carriers and significantly improve the hydrogen evolution efficiency. In this work, we found that g-C3N4 decorated with 1.0 wt% CDs achieved the highest hydrogen evolution rate (2878.2 μmol/h/g) under visible light (λ > 420 nm), which was about 5 times higher than that of pristine g-C3N4 (582.2 μmol/h/g). Schematic illustration of the separation and transfer of photo-generated charge carriers of CDs-g-C3N4 nanoparticles under visible light irradiation.
  • Key Words:CDs G-C3N4 Photocatalytic Water splitting
  • Translation or Not:no